Oslo CTM3

Oslo CTM3 Chemistry : The troposphere

The tropospheric chemistry module
The tropospheric chemistry scheme is run with a numerical time step of 15 minutes (5 minutes for OH/HO2/RO2-reactions), contains 46 species and also some intermediate short lived species treated within chemistry only. The scheme takes into account 86 thermal reactions, 17 photolytic reactions and 2 heterogeneous reactions (which are independent of the stratospheric heterogeneous chemistry). It includes detailed hydrocarbon chemistry and has been thoroughly tested (Berntsen and Isaksen, 1997; Kraabøl et al., 1999; Berglen et al., 2004; Brunner et al., 2003).

The main reference for the tropospheric chemistry is Berntsen and Isaksen (1997).

Tropospheric components
Listed here are all the components in the tropospheric module of the Oslo CTM3, whether they are transported (T=Y) or not (T=N), and also the chemical domain of interest (C): T is troposphere only, and B is both tropopshere and stratosphere. Wet deposition is listed as WD.

Nr Component T/C WD Remarks
01 O3 Y/B Y
04 HNO3 Y/B Y
05 PANx Y/T (PAN+CH3COO2)
06 CO Y/B
07 C2H4 Y/T
08 C2H6 Y/T
09 C3H6 Y/T
10 C4H10 Y/T
11 C6H14 Y/T
12 C6HXR Y/T m-xylene
13 CH2O Y/B Y
14 CH3CHO Y/T Y
15 H2O2 Y/B Y
16 CH3O2H Y/B Y
17 HO2NO2 Y/B Y
18 CH3COY Y/T CH3COCOCH3
19 CH3COX Y/T CH3COC2H5
20 Isoprene Y/T C5H8
21 HO2 Y/B
22 CH3O2 N/B
23 C2H5O2 N/T
24 C4H9O2 N/T
25 C6H13O2 N/T
27 CH3COB N/T CH3COCH(O2)CH3
28 CH3XX N/T CH3CH(O2)CH2OH
29 AR1 N/T first RO2 radical from the reaction of m-xylene + OH
30 AR2 N/T a C-5 carbonyl compound; from the reaction of AR1 + NO
31 AR3 N/T a C-5 RO2 radical; from the reaction of AR2 + OH
32 ISOR1 N/T first RO2 radical from the reaction of isoprene + OH
33 ISOK N/T Y methylvinylketone (MVK) + methacrolein (MACR)
34 ISOR2 N/T RO2 radical formed from MVK+OH or MACR+OH
35 HCOHCO Y/T
36 RCOHCO Y/T
37 CH3X Y/T CH3COO2
38 O(3P) N/B
39 O(1D) N/B
40 OH N/B
41 NO3 Y/B
42 N2O5 Y/B
43 NO Y/B
44 NO2 Y/B
46 CH4 Y/B
48 C3H8 Y/T
49 C3H7O2 Y/T
50 Acetone Y/T CH3C(O)CH3
51 CH3COD Y/T CH3COCH2(O2)
References

Berglen, T. F., T. K. Berntsen, I. S. A. Isaksen, and J. K. Sundet: A global model of the coupled sulfur/oxidant chemistry in the troposphere: The sulfur cycle, J. Geophys. Res., 109(D19310), doi:10.1029/2003JD003948, 2004.

Berntsen, T., and I. S. A. Isaksen: A global 3-D chemical transport model for the troposphere, 1, Model description and CO and Ozone results, J. Geophys. Res., 102(D17), 21239-21280, doi:10.1029/97JD01140, 1997.

Brunner, D.; J. Staehelin, H. L. Rogers, M. O. Köhler, J. A. Pyle, D. Hauglustaine, L. Jourdain, T. K. Berntsen, M. Gauss, I. S. A. Isaksen, E. Meijer, P. van Velthoven, G. Pitari, E. Mancini, V. Grewe, and R. Sausen: An evaluation of the performance of chemistry transport models by comparison with research aircraft observations. Part 1: Concepts and overall model performance. Atmos. Chem. Phys., 3, 1609-1631, doi:10.5194/acp-3-1609-2003, 2003.

Kraabøl, A. G., F. Stordal, P. Konopka, and S. Knudsen: The NILU aircraft plume model: A technical description. Technical Report TR 4/99, Norwegian Institute for Air Research, 1999.

Last modified: Thu May 10 15:38:40 CEST 2012 © Amund Søvde