Introduction



next up previous
Next: Construction of a Up: Construction of a Previous: Construction of a

Introduction

The term "Diffusion Limited Aggregation" (DLA) [1] refers to a simple growth algorithm in which individual particles are added to a growing cluster through a diffusion-like process. Starting from any suitable cluster seed fixed in -dimensional space, a new particle is launched at a random position far away from the cluster and undergoes Brownian motion. When the randomly walking particle contacts the cluster, it is stopped and incorporated to the cluster at its contacting position. This process of launching a random walker and adding it to the cluster on its first contact is repeated until the cluster has reached a desired number of particles (mass), . The DLA model generates strongly ramified clusters with a complex geometry. Figure 1 displays a DLA cluster embedded in two-dimensional space at different stages of growth. The cluster consists of identical discs of diameter . The cluster seed was a single disc.

Due to the non-deterministic nature of Brownian motion, each DLA cluster represents the individual outcome of a statistical process. Although the process itself is simple, its boundary conditions are not. The surface of the cluster constitutes the absorbing boundary for the diffusing particles, and changes while the cluster grows.

More specifically, DLA is a growth process in which the growth rate of the cluster boundary is determined by the gradient of a scalar field that fulfills the Laplace equation. The boundary conditions are that on the cluster boundary, and at infinity. The random walkers provide unbiased samples of the Laplace field , and the probability of contacting the cluster boundary at a given position is proportional to . In summary, DLA is a model for Laplacian growth in the presence of statistical noise.

  
Figure 1: A two-dimensional, off-lattice DLA cluster at six different stages of growth. The cluster consists of identical discs of diameter , and is shown when it contains , , , , , and particles, respectively. The cluster seed was one single disc. According to the finite printer resolution, only a fraction of all particles are shown for in order not to change the visual appearance of the cluster.

Consequently, the DLA algorithm is a relevant model for many Laplacian growth phenomena in nature, including fluid-fluid displacement in Hele-Shaw cells [2] and in porous media [4][3], bacterial growth [5], electrodeposition [7][6], thin film deposits [8], dissolution of porous materials [10][9], and dielectric breakdown [11]. A more extensive discussion of DLA and its relation to natural growth processes may be found in Refs. [12] and [13].

DLA clusters are known to be fractals. To illustrate this we show in Figure 2 the result of a measurement of the average number of particles, , within a distance of a given particle of a DLA cluster. To obtain , particles , were randomly chosen from the first particles of the cluster shown in Fig. 1. When the cluster consisted of particles, the number of particles within distance to particle , , was counted for each of the selected particles. Finally, was calculated as the average value of . For , the relation between and is consistent with the scaling law

Consequently, the particle density, , is not constant, but decreases when increasing the length scale on which the density is measured. This scale dependence of the mass density is apparent in Fig. 1, where larger clusters clearly are more sparse than smaller ones. The scaling exponent can be interpreted as an effective fractal dimensionality of the cluster [14].

  
Figure 2: Log-log plot of average mass within distance to a given particle as a function of for two-dimensional, off-lattice DLA. Filled circles are experimental data, obtained from the DLA cluster shown in Fig. 1 as explained in the text. The line corresponds to the fit , indicating a fractal dimensionality of of the cluster.

From Fig. 2 a fractal dimensionality may be read off, in reasonable agreement with the accepted value of for two-dimensional, off-lattice DLA [15], obtained from the dependence of the cluster radii of gyration on . The two crossover length that define the regime in which the scaling law holds are the particle diameter, , and the radius of the complete cluster of particles, , respectively.



next up previous
Next: Construction of a Up: Construction of a Previous: Construction of a



Thomas Walmann
Wed Mar 13 12:19:50 MET 1996